Stretchable electronics are a new, emerging class of electronic devices that can conform to complex non-planar and deformable surfaces such as human organs, textiles, and robotics. Functional fillers incorporated with elastic polymers form composites for use in intrinsically stretchable electronics. These composites can be amenable to high-throughput, low-cost, additive printing technologies that include screen, inkjet, flexography, and 3D printing. However, the properties of the functional and elastic materials used to date have been mutually antagonistic, thus limiting achievement of state-of-the-art functional properties and high elasticity. The present invention relates to the development of random composite inks using triblock copolymer for stretchable electronics. The key novelty offered here is the ability to tolerate higher loadings of inelastic, functional materials without sacrificing the elastic properties of the ink.